|
|
wt/vol
|
MW/conc.
|
moles
|
density
|
equivs.
|
yield
|
|
I
|
0.156 g
|
208.25
|
0.0007
|
|
1.0
|
|
|
II
|
0.81 mL
|
1.0 M
|
0.0008
|
|
1.1
|
|
|
III
|
6.75 mL
|
-
|
-
|
|
|
|
|
IV
|
2.25 mL
|
-
|
-
|
|
|
|
|
V
|
0.112 g
|
164.20
|
0.0007
|
|
|
(91%)
|
Procedure: 50 mL
1-neck flask, stirbar, septum, N2 inlet
Dissolved
0.156 g of ester I in 6.75 mL of
hexanes and 2.25 mL of dry Et2O. Stirred; cooled to -78 C. Added 0.81 mL DIBAL (1.0 M in hexanes). After 10 min, the reaction was quenched
with MeOH. Added ~10 mL of sat.
aq. Na/K tartrate, stirred 30 min
and extracted with Et2O. The organic layer was dried over MgSO4, filtered
and the solvent was removed by rotary evaporation. The product was isolated by flash chromatography on silica
gel using 10:90 EtOAc-hexanes as eluant.
The product was a clear, colorless oil.