|
|
wt/vol
|
MW
|
moles
|
density
|
equivs.
|
yield
|
|
I
|
2.46 mL
|
56.06
|
0.0423
|
0.963
|
1.0
|
|
|
II
|
1.114 g
|
24.00
|
0.0464
|
|
1.1
|
|
|
III
|
5.20 mL
|
171.04
|
0.0437
|
1.438
|
1.0
|
|
|
IV
|
40 mL
|
-
|
-
|
|
|
|
|
V
|
6.166 g
|
146.18
|
0.0422
|
|
|
(100%)
|
Procedure: 100 mL
1-neck flask, stirbar, septum, N2 inlet
Prepared
a suspension of 1.114 g of powdered NaH in 40 mL of dry THF. Stirred; cooled to 0 C. Added 2.46 mL of propargyl alcohol
dropwise. Hydrogen gas evolution
occurred. Stirred for 15 min. Added 5.20 mL of BnBr. and allowed the reaction mixture to
slowly warm to rt. After 24 h the
reaction was quenched with sat. aq. NH4Cl and extracted with Et2O. The organic layer was dried over MgSO4,
filtered and the solvent was removed by rotary evaporation. The product was isolated by Kugelrohr
distillation (15 mm, 100 C) as a clear, colorless oil.
notes
This reaction is a simple SN2
substitution with in situ formed alkoxide displacing bromine.